Lightweight Flexible Polyimide-Derived Laser-Induced Graphenes for High-Performance Thermal Management Applications
出版日期:2022-08-18 00:00:00
著者:Yu-Sheng Hsiao; Cai-Wan Chang-Jian; Tzu-Yen Huang; Ying-Lin Chen; Chung-Wei Huang; Jen-Hsien Huang; Nian-Jheng Wu; Shih-Chieh Hsu; Chih-Ping Cheng
著錄名稱、卷期、頁數:Chemical Engineering Journal 451(Part 2), 138656
摘要:Laser pyrolysis of polyimide (PI) is a promising approach for preparing porous graphenes with hierarchical structures. In this study, we used a dual-focusing lens with a collimator to generate a highly concentrated CO2 laser beam with a high focal energy density. The resulting PI-derived graphene (PIDG) obtained under high-intensity laser irradiation possessed a high degree of graphitization, a low sheet resistance (27.4 Ω/sq.), and a large surface area (240.4 m2/g). Through optimization of the high-intensity laser parameters, we obtained a hierarchical PIDG possessing a fiber-like structure. We used this PIDG as a flexible heater and efficient heat sink for Si photovoltaic (PV) and light-emitting diode (LED) modules. The developed heater could reach a temperature of 202.6 °C under an applied voltage of 16 V, with rapid responses and remarkable flexibility. As a result of improved convective and radiative heat dissipation, the PIDG-based heat sink lowered the operating temperatures of the Si PV and LED modules efficiently. Accordingly, the power conversion efficiency of the Si PV and the lifetime of the LED module both increased dramatically.
關鍵字:Graphene; CO2 laser; Nanofiber structure; Electrothermal heater; Heat dissipation
語言:en_US
ISSN:1385-8947; 1873-3212
期刊性質:國外
收錄於:SCI
審稿制度:否
國別:NLD
出版型式:電子版,紙本